Pufnstuf

Freddy the Flute / Googy Gopher / Orson Vulture (voice)

Googy Gopher / Orville Pelican

Miss Flick

Dowager Tree / Granddaughter Clock (voice)

Dr. Blinky / Ludicrous Lion

Seymore Spider / Clang

Witchiepoo

Witch Hazel (as Mama Cass)

Dr. Blinky / Ludicrous Lion / Seymore Spider / Various (voice)

Jimmy

Boss Witch

Shirley Pufnstuf

H. R. Pufnstuf / Henrich Rat / Living Island Boat / Orville Pelican / Polka-Dotted Horse / Stupid Bat / West Wind (voice) (as Al Melvin)

Polkadotted Horse